Stephen Toth’s favorite structure is:

Haemoglobin

Haemoglobin

Source: http://www.wellcomecollection.org/whats-on/exhibitions/from-atoms-to-patterns/image-galleries/x-ray-crystallography.aspx

Why?

Hemoglobin is my favorite because I draw Hemoglobin every other weekend for my job at the hospital and it has been nothing but fun and sometimes challenging (some patients are hard sticks). —Stephen Toth

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